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bioaccumulations based on a global data set and the implications for aquatic systems with aggravating nutrient

《环境科学与工程前沿（英文）》 2022年 第16卷 第3期 doi: 10.1007/s11783-021-1471-x

摘要：

• Hg bioaccumulation by phytoplankton varies among aquatic ecosystems.

关键词： Plankton     Hg bioaccumulation     Physiological characteristics     A cross-system analysis     Nutrient compositions     Global data set    

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NO conversion by positive streamer discharge—effects of gas compositions and reaction conditions

HE Wei, ZHU Tianle, LI Jing

《环境科学与工程前沿（英文）》 2007年 第1卷 第2期   页码 153-158 doi: 10.1007/s11783-007-0027-z

摘要： The effects of gas compositions and reaction conditions on NO conversion by positive streamer discharge were experimentally investigated by using a link tooth wheel-cylinder reactor. The results showed that NO conversion increased w

关键词： conversion     streamer discharge     wheel-cylinder     positive streamer    

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Octane compositions in sulfuric acid catalyzed isobutane/butene alkylation products: experimental and

Lina Liang, Youzhi Liu, Weizhou Jiao, Qiaoling Zhang, Chao Zhang

《化学科学与工程前沿（英文）》 2021年 第15卷 第5期   页码 1229-1242 doi: 10.1007/s11705-020-2030-x

摘要： Octanes in alkylation products obtained from industrial alkylation were studied by batch experiments. More than eight octane isomers were identified and quantified by gas chromatography-mass spectrometry. Based on a classic carbenium ion mechanism, the carbocation transition states in concentrated sulfuric acid catalyzed alkylation were investigated using quantum-chemical simulations and predicted the concentration and octane isomerization products including trimethylpentane and dimethylhexane as well as the formation of heavier compounds that resulted from the oligomerization of octane and butene. The agreement between model calculations and experimental data was quite satisfactory. Calculation results indicated that composition and content of trimethylpentanes in the alkylation products were 2,2,4-trimethylpentane>2,3,3-trimethylpentane>2,3,4-trimethylpentane>2,2,3-trimethylpentane whether the 2-butene or -butene acts as olefin. Heavier compounds in the alkylate were primarily formed by the oligomerization of dimethylhexane with 1-butene. Hopefully, the carbocation transition state models developed in this work will be useful for understanding the product distributions of octane in alkylation products.

关键词： sulfuric acid catalyzed alkylation     carbocation reaction     transition state     octane compositions    

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Managing nutrient for both food security and environmental sustainability in China: an experiment for

Fusuo ZHANG, Zhenling CUI, Weifeng ZHANG

《农业科学与工程前沿（英文）》 2014年 第1卷 第1期   页码 53-61 doi: 10.15302/J-FASE-2014006

摘要： The challenges of how to simultaneously ensure global food security, improve nitrogen use efficiency (NUE) and protect the environment have received increasing attention. However, the dominant agricultural paradigm still considers high yield and reducing environmental impacts to be in conflict with one another. Here we examine a Three-Step-Strategy of past 20 years to produce more with less in China, showing that tremendous progress has been made to reduce N fertilizer input without sacrificing crop yield. The first step is to use technology for in-season root-zone nutrient management to significantly increase NUE. The second is to use technology for integrated nutrient management to increase both yield and NUE by 15%–20%. The third step is to use technology for integrated soil-crop system management to increase yield and NUE by 30%–50% simultaneously. These advances can thus be considered an effective agricultural paradigm to ensure food security, while increasing NUE and improving environmental quality.

关键词： integrated nutrient management     integrated soil-crop system management     environmental protection     food security     resource use efficiency    

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Predicting the elemental compositions of solid waste using ATR-FTIR and machine learning

《环境科学与工程前沿（英文）》 2023年 第17卷 第10期 doi: 10.1007/s11783-023-1721-1

摘要：

● A method based on ATR-FTIR and ML was developed to predict CHNS contents in waste.

关键词： Elemental composition     Infrared spectroscopy     Machine learning     Moisture interference     Solid waste     Spectral noise    

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Dynamic changes of protein corona compositions on the surface of zinc oxide nanoparticle in cell culture

Vo-Van Giau, Yoon-Hee Park, Kyu-Hwan Shim, Sang-Wook Son, Seong-Soo A. An

《化学科学与工程前沿（英文）》 2019年 第13卷 第1期   页码 90-97 doi: 10.1007/s11705-018-1766-z

摘要：

The potential applications of nanomaterials used in nanomedicine as ingredients in drug delivery systems and in other products continue to expand. When nanomaterials are introduced into physiological environments and driven by energetics, they readily associate proteins forming a protein corona (PC) on their surface. This PC could result in an alteration of the nanomaterial’s surface characteristics, affecting their interaction with cells due to conformational changes in adsorbed protein molecules. However, our current understanding of nanobiological interactions is still very limited. Utilizing a liquid chromatography–mass spectroscopy/mass spectroscopy technology and a Cytoscape plugin (ClueGO) approach, we examined the composition of the PC for a set of zinc oxide nanoparticles (ZnONP) from cell culture media typically and further analyzed the biological interaction of identified proteins, respectively. In total, 36 and 33 common proteins were investigated as being bound to ZnONP at 5 min and 60 min, respectively. These proteins were further analyzed with ClueGO, a Cytoscape plugin, which provided gene ontology and the biological interaction processes of identified proteins. Proteins bound to the surface of nanoparticles that may modify the structure, therefore the function of the adsorbed protein could be consequently affect the complicated biological processes.

关键词： ZnONPs     nanoparticles     protein corona     ClueGO    

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HOTSPOTS OF NUTRIENT LOSSES TO AIR AND WATER: AN INTEGRATED MODELING APPROACH FOR EUROPEAN RIVER BASINS

《农业科学与工程前沿（英文）》 2023年 第10卷 第4期   页码 579-592 doi: 10.15302/J-FASE-2023526

摘要：

Nutrient pollution of air and water is a persistent problem in Europe. However, the pollution sources are often analyzed separately, preventing the formulation of integrative solutions. This study aimed to quantify the contribution of agriculture to air, river and coastal water pollution by nutrients. A new MARINA-Nutrients model was developed for Europe to calculate inputs of nitrogen (N) and phosphorus (P) to land and rivers, N emissions to air, and nutrient export to seas by river basins. Under current practice, inputs of N and P to land were 34.4 and 1.8 Tg·yr–1, respectively. However, only 12% of N and 3% of P reached the rivers. Agriculture was responsible for 55% of N and sewage for 67% of P in rivers. Reactive N emissions to air from agriculture were calculated at 4.0 Tg·yr–1. Almost two-fifths of N emissions to air were from animal housing and storage. Nearly a third of the basin area was considered as pollution hotspots and generated over half of N emissions to air and nutrient pollution in rivers. Over 25% of river export of N ended up in the Atlantic Ocean and of P in the Mediterranean Sea. These results could support environmental policies to reduce both air and water pollution simultaneously, and avoid pollution swapping.

关键词： agriculture     air-water modeling     European rivers     nutrient pollution     sewage systems     source attribution    

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Unintended nutrient imbalance induced by wastewater effluent inputs to receiving water and its ecological

《环境科学与工程前沿（英文）》 2022年 第16卷 第11期 doi: 10.1007/s11783-022-1584-x

摘要： Eutrophication is the most widespread water quality issue globally. To date, most efforts to control eutrophication have focused on reductions of external nutrient inputs, yet importance of nutrient stoichiometry and subsequent shift in plankton composition in aquatic ecosystem has been largely neglected. To address eutrophication, improved sanitation is one of the United Nations Sustainable Development Goals, spurring the constructions of wastewater treatment facilities that have improved water quality in many lakes and rivers. However, control measures are often targeted at and effective in removing a single nutrient from sewage and thus are less effective in removing the others, resulting in the changes of nutrient stoichiometry. In general, more effective phosphorus removal relative to nitrogen has occurred in wastewater treatment leading to substantial increases in N/P ratios in effluent relative to the influent. Unfortunately, high N/P ratios in receiving waters can impose negative influences on ecosystems. Thus, long-term strategies for domestic wastewater management should not merely focus on the total reduction of nutrient discharge but also consider their stoichiometric balances in receiving waters.

关键词： Nutrient stoichiometry     Wastewater treatment     Ecosystem functioning     Water quality management    

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MANURE AND METROPOLES---A GLOBAL FRAMEWORK FOR NUTRIENT CYCLING IN FOOD SYSTEMS

《农业科学与工程前沿（英文）》 2021年 第8卷 第1期

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Pelagic-benthic coupling of the microbial food web modifies nutrient cycles along a cascade-dammed river

《环境科学与工程前沿（英文）》 2022年 第16卷 第4期 doi: 10.1007/s11783-021-1484-5

摘要：

• Structure of multi-trophic microbial groups were analyzed using DNA metabarcoding.

关键词： Reservoir     Multi-trophic     Beta diversity     Predator-prey     Nutrient accumulation    

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Insights into the changes of amino acids, microbial community, and enzymatic activities related with the nutrient

《环境科学与工程前沿（英文）》 2023年 第17卷 第3期 doi: 10.1007/s11783-023-1635-y

摘要：

● The highest seed germination index was achieved at 0.3 g/g total solids of food waste.

关键词： Composting     Food waste     Amino acids     Microbial community     Enzymatic activity     Nutrient quality    

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Effects of riparian vegetation patterns on the distribution and potential loss of soil nutrients: a case study of the Wenyu River in Beijing

Erhui GUO,Liding CHEN,Ranhao SUN,Zhaoming WANG

《环境科学与工程前沿（英文）》 2015年 第9卷 第2期   页码 279-287 doi: 10.1007/s11783-014-0667-8

摘要： A riparian ecosystem is an ecological transition zone between a river channel and terrestrial ecosystems. Riparian ecosystems play a vital role in maintaining stream health and bank stabilization. The types of riparian vegetation have changed greatly because of human activities along the Wenyu River. This study examines the impact of riparian vegetation patterns on water pollution due to soil nutrient loss. Four riparian vegetation patterns from the river channel to the upland were chosen as the focus of this study: grassland, cropland, grassland-cropland, and grassland-manmade lawn. The different distributions of soil nutrients along vegetation patterns and the potential risk of nutrient loss were observed and compared. The results showed that riparian cropland has the lowest value of total nitrogen (TN), total phosphorus (TP), available nitrogen (AN), available phosphorus (AP), and organic matter (OM), but it has the highest soil bulk density (BD). The distributions of soil TN, TP, AN, AP, and OM exhibited a declining trend from the upland toward the river channel for riparian cropland, whereas a different trend was observed for the riparian grassland. The vegetation patterns of grassland-cropland and grassland-manmade lawn show that the grassland in the lower slope has more nutrients and OM but lower soil BD than the cropland or manmade lawn in the upper slope. So, the lower-slope grassland may intercept and infiltrate surface runoff from the upland. The lower-slope grassland has higher levels of soil TN, TP, AN, and AP, and thus it may become a new source of nutrient loss. Our results suggest that the management of the riparian vegetation should be improved, particularly in densely populated areas, to control soil erosion and river pollution.

关键词： riparian     vegetation patterns     soil nutrient distribution     nutrient loss     management    

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Simulation of long-term nutrient removal in a full-scale closed-loop bioreactor for sewage treatment:

Zheng LI,Rong QI,Wei AN,Takashi MINO,Tadashi SHOJI,Willy VERSTRAETE,Jian GU,Shengtao LI,Shiwei XU,Min YANG

《环境科学与工程前沿（英文）》 2015年 第9卷 第3期   页码 534-544 doi: 10.1007/s11783-014-0660-2

摘要： In this study, the performance of nitrogen and phosphorus removal in a full-scale closed-loop bioreactor (oxidation ditch) system was simulated using the ASM2d model. Routine data describing the process for two years were compiled for calibration and validation. To overcome the identifiability problem, the classic Bayesian inference approach was utilized for parameter estimation. The calibrated model could describe the long-term trend of nutrient removal and short-term variations of the process performance, showing that the Bayesian method was a reliable and useful tool for the parameter estimation of the activated sludge models. The anoxic phosphate uptake by polyphosphate accumulating organisms (PAO) contributed 71.2% of the total Poly-P storage, which reveals the dominance of denitrifying phosphorus removal process under the oxygen limiting conditions. It was found that 58.7% of the anoxic Poly-P storage and denitrification by PAO in the reactor was achieved in the aerated compartment, implying that the PAO’s anoxic activity was significantly stimulated by the low dissolved oxygen (DO) level in this compartment due to the oxygen gradient caused by brush aerator.

关键词： activated sludge model     Bayesian inference     biological nutrient removal     closed-loop bioreactor     oxidation ditch     denitrifying polyphosphate accumulating organisms    

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Water---- and nutrient and energy---- systems in urbanizing watersheds

Rodrigo VILLARROEL WALKER, Michael Bruce BECK, Jim W. HALL

《环境科学与工程前沿（英文）》 2012年 第6卷 第5期   页码 596-611 doi: 10.1007/s11783-012-0445-4

摘要： Driven by considerations of sustainability, it has become increasingly difficult over the past 15–20 years — at least intellectually — to separate out the water infrastructure and water metabolism of cities from their intimately inter-related nutrient and energy metabolisms. Much of the focus of this difficulty settles on the wastewater component of the city’s water infrastructure and its associated fluxes of nutrients (N, P, C, and so on). Indeed, notwithstanding the massive volumes of these materials flowing into and out of the city, the notion of an urban nutrient infrastructure is conspicuous by its absence. Likewise, we do not tend to discuss, or conduct research into, “soilshed” agencies, or soilshed management, or Integrated Nutrient Resources Management (as opposed to its most familiar companion, Integrated Water Resources Management, or IWRM). The paper summarizes some of the benefits (and challenges) deriving from adopting this broader, multi-sectoral “systems” perspective on addressing water-nutrient-energy systems in city-watershed settings. Such a perspective resonates with the growing interest in broader policy circles in what is called the “water-food-energy security nexus”. The benefits and challenges of our Multi-sectoral Systems Analysis (MSA) are illustrated through computational results from two primary case studies: Atlanta, Georgia, USA; and London, UK. Since our work is part of the International Network on Cities as Forces for Good in the Environment (CFG; see www.cfgnet.org), in which other case studies are currently being initiated — for example, on Kathmandu, Nepal — we close by reflecting upon these issues of water-nutrient-energy systems in three urban settings with quite different styles and speeds of development.

关键词： cities     climate change     energy sector     nutrient sector     systems analysis     resource recovery     water-food-energy security    

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Mass loss and nutrient dynamics during litter decomposition in response to warming and nitrogen addition

Haiyan REN, Jie QIN, Baolong YAN, Alata, Baoyinhexige, Guodong HAN

《农业科学与工程前沿（英文）》 2018年 第5卷 第1期   页码 64-70 doi: 10.15302/J-FASE-2017194

摘要： Plant litter decomposition has been studied extensively in the context of both warming and increased atmospheric nitrogen deposition. However, the temporal patterns of mass loss and nutrient release in response to warming and nitrogen addition remain unclear. A 2-year decomposition experiment aimed to examine the effects of warming and nitrogen addition on decomposition rate, and nitrogen and phosphorus dynamics. The effects of warming and nitrogen addition on decomposition of litter of , a dominant species in a desert steppe of northern China, were studied. Warming and nitrogen addition significantly enhanced litter mass loss by 10% and 16%, respectively, and moreover promoted nitrogen and phosphorus release from the litter in the first year of decomposition, followed by an immobilization period. The interactive effects of warming and nitrogen addition on mass loss, nitrogen and phosphorus concentrations of litter were also found during the decomposition. This study indicates that warming and nitrogen addition increased litter mass loss through altering litter quality. These findings highlight that interactions between climate change and other global change factors could be highly important in driving decomposition responses.

关键词： climate warming     grassland     litter decomposition     nitrogen deposition     nutrient release    

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标题 作者 时间 类型 操作

bioaccumulations based on a global data set and the implications for aquatic systems with aggravating nutrient

期刊论文

NO conversion by positive streamer discharge—effects of gas compositions and reaction conditions

HE Wei, ZHU Tianle, LI Jing

期刊论文

Octane compositions in sulfuric acid catalyzed isobutane/butene alkylation products: experimental and

Lina Liang, Youzhi Liu, Weizhou Jiao, Qiaoling Zhang, Chao Zhang

期刊论文

Managing nutrient for both food security and environmental sustainability in China: an experiment for

Fusuo ZHANG, Zhenling CUI, Weifeng ZHANG

期刊论文

Predicting the elemental compositions of solid waste using ATR-FTIR and machine learning

期刊论文

Dynamic changes of protein corona compositions on the surface of zinc oxide nanoparticle in cell culture

Vo-Van Giau, Yoon-Hee Park, Kyu-Hwan Shim, Sang-Wook Son, Seong-Soo A. An

期刊论文

HOTSPOTS OF NUTRIENT LOSSES TO AIR AND WATER: AN INTEGRATED MODELING APPROACH FOR EUROPEAN RIVER BASINS

期刊论文

Unintended nutrient imbalance induced by wastewater effluent inputs to receiving water and its ecological

期刊论文

MANURE AND METROPOLES---A GLOBAL FRAMEWORK FOR NUTRIENT CYCLING IN FOOD SYSTEMS

期刊论文

Pelagic-benthic coupling of the microbial food web modifies nutrient cycles along a cascade-dammed river

期刊论文

Insights into the changes of amino acids, microbial community, and enzymatic activities related with the nutrient

期刊论文

Effects of riparian vegetation patterns on the distribution and potential loss of soil nutrients: a case study of the Wenyu River in Beijing

Erhui GUO,Liding CHEN,Ranhao SUN,Zhaoming WANG

期刊论文

Simulation of long-term nutrient removal in a full-scale closed-loop bioreactor for sewage treatment:

Zheng LI,Rong QI,Wei AN,Takashi MINO,Tadashi SHOJI,Willy VERSTRAETE,Jian GU,Shengtao LI,Shiwei XU,Min YANG

期刊论文

Water---- and nutrient and energy---- systems in urbanizing watersheds

Rodrigo VILLARROEL WALKER, Michael Bruce BECK, Jim W. HALL

期刊论文

Mass loss and nutrient dynamics during litter decomposition in response to warming and nitrogen addition

Haiyan REN, Jie QIN, Baolong YAN, Alata, Baoyinhexige, Guodong HAN

期刊论文